Correlations between Photons in Resonance Fluorescence Emitted by an Atom Near a Metal Surface.

Abstract

The photon correlations of resonance fluorescence emitted by a degenerate two-level atom near a metal surface are studied. An intense non monochromatic optical laser drives a low lying atomic transition, and the emitted fluorescence is detected by a photon counter. An expression for the spontaneous decay operator is derived, and it appears that the various substates of the upper level have a different lifetime due to the presence of the surface, or equivalently, due to the loss of spherical symmetry. The temporal photon correlation function is then evaluated in terms of a photon-emission operator and the time evolution operator for the atomic density matrix. The general theory is exemplified with a detailed elaboration of the j sub g = 0 yields j sub e = 1 transition, for which the two-photon correlation is obtained explicitly as a function of the lifetime A(h), depending on the atom surface distance h, the laser linewidth, the detuning from resonance, and the dipole-coupling strength with the external field. Keywords: Photon correlations; Resonance fluorescence; Atom near metal surface; Loss of spherical symmetry; Substates; Different lifetimes.

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Document Details

Document Type
Technical Report
Publication Date
Oct 01, 1987
Accession Number
ADA188365

Entities

People

  • Henk F. Arnoldus
  • Thomas F. George

Organizations

  • University at Buffalo

Tags

Communities of Interest

  • Air Platforms
  • Weapons Technologies

DTIC Thesaurus Topics

  • Abstracts
  • Air Force
  • Chemical Engineering
  • Chemistry
  • Circular Polarization
  • Differential Equations
  • Frequency
  • Governments
  • Lasers
  • Linear Polarization
  • Materials
  • Materials Science
  • Military Research
  • New York
  • Standards
  • United States
  • United States Government

Fields of Study

  • Physics

Readers

  • Molecular Photonics/Laser Physics
  • Quantum spin resonance or Electron Paramagnetic Resonance spectroscopy.

Technology Areas

  • Directed Energy
  • Directed Energy - Lasers