Advanced B and Al Iota Combustion Kinetics over Wide Temperature Ranges.

Abstract

Current ability to improve the combustion efficiency of B and Al solid propellants and slurries is hampered by a lack of understanding and knowledge of the kinetics of the individual reactions involved and the ways and manner by which temperature affects the rate coefficients and product channels. While the simple Arrhenius-type equation k(T) = AT(to the 1/2 power) exp(-E(A)/RT) has over limited temperature ranges been of great value, when applied to wide temperature ranges it is often not obeyed. Particularly for exothermic and slightly endothermic reactions, order of magnitude errors can be made by extrapolations based on the Arrhenius equation. It is the goal of this program to provide an insight in the kinetic behavior of B and Al radical oxidation reactions as influenced by temperature. To this end measurements are made in high-temperature fast-flow reactors (HTFFR). These unique tools provide measurements on isolated elementary reactions in a heat bath.

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Document Details

Document Type
Technical Report
Publication Date
Dec 17, 1987
Accession Number
ADA190752

Entities

People

  • Arthur Fontijn

Organizations

  • Rensselaer Polytechnic Institute

Tags

Communities of Interest

  • Human Systems
  • Weapons Technologies

DTIC Thesaurus Topics

  • Arrhenius Equation
  • Chemical Compounds
  • Chemical Kinetics
  • Chemical Reactions
  • Chemistry
  • Combustion
  • Elements
  • Endothermic Reactions
  • Equations
  • High Temperature
  • Kinetics
  • Laser Induced Fluorescence
  • Molecules
  • Oxidation
  • Physics
  • Solid Propellants
  • Spectrometers

Readers

  • Combustion science or combustion engineering.
  • Systems Analysis and Design