ArF Laser Photoproduction and Sensitive Detection of Carbon Atoms from Simple Fuel Molecules.

Abstract

Excimer lasers are currently being used as a means of photofragmentation and fragment excitation for chemical detection purposes, as well as for activation of reactive mixtures. In the case of small fuel molecules, this phenomenon is generally poorly understood and needs to be studied further. This report, therefore, describes experiments aimed at a better understanding of the interaction of simple carbon-containing fuel molecules with the ArF excimer laser, particularly with respect to potential analytical applications. Such an application, for instance, would be for a gas chromatographic detector of propellant pyrolysis products. Specifically, in this report we describe experiments where carbon atoms were generated by multiphoton photolysis of CO, CH4, C22, C3H8, CH3OH and CH3COCH3 using the ArF (193 nm) laser. Keywords: Carbon monoxide, Methane, Acetylene, Propane, Carbinols, Acetone.

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Document Details

Document Type
Technical Report
Publication Date
Apr 01, 1987
Accession Number
ADA191684

Entities

People

  • Andrzej W. Miziolek
  • Angelo J. Alfano
  • Rosario C. Sausa

Organizations

  • Ballistic Research Laboratory

Tags

Communities of Interest

  • Energy and Power Technologies
  • Materials and Manufacturing Processes
  • Space
  • Weapons Technologies

DTIC Thesaurus Topics

  • Chemical Detection
  • Chemistry
  • Classification
  • Detection
  • Detectors
  • Dye Lasers
  • Excimer Lasers
  • Fluorescence
  • Ionization
  • Jet Propulsion
  • Laser Applications
  • Laser Beams
  • Laser Induced Fluorescence
  • Lasers
  • Military Research
  • Molecules
  • Ultraviolet Lasers

Fields of Study

  • Physics

Readers

  • Molecular Photonics/Laser Physics
  • Organic Chemistry

Technology Areas

  • Directed Energy