A Methodology for Characterizing Reactive Coatings: Time-Temperature-Transformation (TTT) Analysis of the Competition Between Cure, Evaporation and Thermal Degradation for an Epoxy-Phenolic System

Abstract

A methodology, in terms of a macroscopic isothermal time-temperature- transformation (TTT) diagram, is presented for characterizing the changes which occur isothermally in a reactive thermosetting system in which evaporation, cure, and thermal degradation occur. Iso-weight loss contours show the progress of the loss of volatile material (mostly solvent). The gelation contour corresponds to the macroscopic viscosity rising to a definite level. The vitrification contour corresponds to the glass transition temperature (T sub g) rising to the temperature of cure. Iso-T sub g contours show the progress of cure in terms of the easily measured T sub g (rather than chemical conversion). The iso-T sub g contours also show the influence of thermal degradation competing with cure. Degradation is responsible for difficulties in assigning the glass transition temperature of the fully cured material. Keywords: Epoxy resins, Phenolic plastics, Plastic coatings.

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Document Details

Document Type
Technical Report
Publication Date
Jun 01, 1988
Accession Number
ADA197254

Entities

People

  • John K. Gillham
  • R. B. Prime
  • S. Gan

Organizations

  • Princeton University

Tags

Communities of Interest

  • Energy and Power Technologies

DTIC Thesaurus Topics

  • Body Weight
  • Chemical Engineering
  • Chemistry
  • Coatings
  • Competition
  • Diagrams
  • Energy
  • Engineering
  • Equations
  • Evaporation
  • Glass Transition Temperature
  • Heat Of Activation
  • Military Research
  • Plastics
  • Resins
  • Transition Temperature
  • Transitions

Readers

  • Materials Science and Engineering.
  • Polymer Science and Engineering.