Phosphorus-Containing Derivatives of Decaboranes(14) as Precursors of Boron-Containing Materials

Abstract

Ceramic materials whose properties are attractive for high technology applications often fail to realize their full potential of usefulness due to an inability to be fabricated into complex, durable shapes. One such class of materials is that of the boron-containing ceramics, e.g., boron carbide, boron nitride, boron phosphides, aluminum boride, and boron silicides. We now report the results of an effort to extend the use of preceramic polymers to boron- containing materials. The motivation for this work was to utilize processable materials which give, in general, boron carbide as the major ceramic phase upon pyrolysis. A route to soluble boron-containing polymers has been developed. The synthesis and characterization of phosphorus-containing monomeric and polymeric derivatives of decaborane (B10H14) are given. Preparation and characterization of boron-containing ceramic materials from these molecular and macromolecular species are discussed. Success has been achieved in the areas of ceramic fiber and monolith production and in the area of binder applications for composites of advanced ceramic materials.

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Document Details

Document Type
Technical Report
Publication Date
Jun 25, 1988
Accession Number
ADA197415

Entities

People

  • Dietmar Seyferth
  • William S. Rees Jr.

Organizations

  • Massachusetts Institute of Technology

Tags

Communities of Interest

  • Advanced Electronics
  • Weapons Technologies

DTIC Thesaurus Topics

  • Abrasives
  • Boron Carbides
  • Ceramic Fibers
  • Ceramic Materials
  • Chemical Synthesis
  • Chemistry
  • Composite Materials
  • Inorganic Chemistry
  • Lewis Bases
  • Materials
  • Materials Laboratories
  • Materials Processing
  • Materials Science
  • Military Research
  • Silicon Carbide
  • Technical Ceramics
  • United States

Fields of Study

  • Materials science

Readers

  • Organic Chemistry
  • Reinforced Composite Materials