HgI2 Near-Bandgap Photoluminescence Structure and Its Relationship to Nuclear Detector Quality

Abstract

Mercuric iodide is of interest because it is a high-Z material suitable for applications in nuclear radiation detection. It has an advantage over the more commonly used silicon and germanium detectors in that, with its larger bandgap, it can be operated at room temperature. However, several problems exist in using it for fabricating nuclear detectors, an outstanding one being process control during fabrication. The low-temperature photoluminescence spectra of several mercuric iodide detectors and off-stoichiometric bulk material have been characterized. Phonon energies have been determined with Raman spectroscopy over a range of temperatures. In earlier work some of the near-bandgap photoluminescence features were identified as phonon replicas. After careful examination of Raman and photoluminescence data, we find that one or perhaps more of these features are probably due to shallow electronic levels related to native defects. Suggestions as to the relationship between photoluminescence peaks and detector quality are made.

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Document Details

Document Type
Technical Report
Publication Date
Apr 01, 1988
Accession Number
ADA197515

Entities

People

  • C. Ortale
  • D. Wong
  • L. Van Den Berg
  • R. B. James
  • T. E. Schlesinger

Organizations

  • Sandia National Laboratories

Tags

DTIC Thesaurus Topics

  • Band Gaps
  • Band Structures
  • Bulk Materials
  • Calorific Value
  • Crystal Growth
  • Detectors
  • Energy Bands
  • Engineering
  • Fabrication
  • Jet Propulsion
  • Lasers
  • Low Temperature
  • Nuclear Radiation
  • Radiation
  • Raman Scattering
  • Spectra
  • Spectroscopy

Fields of Study

  • Materials science

Readers

  • Nanoscale Plasmonic Nanotechnology
  • Powder metallurgy of Titanium alloys.
  • Systems Analysis and Design

Technology Areas

  • Microelectronics