High-Pressure Electrochemical Oxidation of Benzene at a Lead Dioxide Electrode in Aqueous Bisulfate Solutions at 25 to 250 deg C

Abstract

The oxidation of benzene at a lead dioxide electrode which produces predominantly benzoquinone, maleic acid, and carbon dioxide, has been investigated in aqueous NaHSO4 solutions as a function of temperature up to 250 deg C. An increase in the benzene concentration does not increase the concentration of benzoquinone formed at high temperature, which is different from the behavior at 25 deg C. The formation of biphenyl at high temperature was also discovered. A novel type of single-pass flow reactor for studying high temperature electrochemistry is described.

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Document Details

Document Type
Technical Report
Publication Date
Dec 01, 1987
Accession Number
ADA198503

Entities

People

  • Allen J. Bard
  • Keith P. Johnston
  • William M. Flarsheim

Organizations

  • University of Texas at Austin

Tags

Communities of Interest

  • Advanced Electronics
  • Energy and Power Technologies

DTIC Thesaurus Topics

  • Alkenes
  • Carbon Dioxide
  • Chemical Reaction Properties
  • Chemical Reactions
  • Chemical Synthesis
  • Chemistry
  • Electrochemical Reactions
  • Electrodes
  • Electrolytes
  • High Pressure
  • High Temperature
  • Hydroxides
  • Measurement
  • Military Research
  • Photoelectrochemical Cells
  • Solubility
  • Water

Fields of Study

  • Chemistry

Readers

  • Electrochemical Surface Science
  • Organic Chemistry
  • Polymer Science and Engineering.