An Electrochemical and Spectroelectrochemical Study of Substituted Alkylidenecyclopropabenzenes. 1-(Diphenylmethylene)cyclopropabenzene in the First Anodic and Cathodic Voltammetric Waves in Acetonitrile

Abstract

Electrochemical and modulated specular reflectance spectroelectrochemical (MSRS) investigations were performed on 1- (diphenylmethylene)cyclopropabenzene in nominally dry acetonitrile solution. The results indicate the formation of a stable anion radical and a quasi stable cation radical. The first order homogeneous rate constant for the decay of the cation radical was computed. Cycloproparenes possess some of the highest strain energies known; the parent compound I has a strain energy of 68 kcal/mol. As a result, the electrochemical oxidation and reduction potentials of the neutral molecules are lower than those of most other electroactive hydrocarbons.

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Document Details

Document Type
Technical Report
Publication Date
Jul 15, 1988
Accession Number
ADA200308

Entities

People

  • B. Halton
  • F. Safarazi
  • J. K. Foley
  • K. Ashley
  • P. J. Stang
  • Q. Mei
  • S. J. Buckland
  • Stanley Pons

Organizations

  • University of Utah

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Communities of Interest

  • Energy and Power Technologies
  • Weapons Technologies

DTIC Thesaurus Topics

  • Abstracts
  • Air Force
  • Alkanes
  • Aromatic Hydrocarbons
  • Chemical Reactions
  • Chemical Synthesis
  • Chemistry
  • Electrochemical Reactions
  • Electrochemistry
  • Electron Transfer
  • Materials
  • Military Research
  • New York
  • Organic Chemistry
  • Square Roots
  • United States
  • Universities

Fields of Study

  • Chemistry

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  • Electrochemical Engineering/ Fuel Cell Technologies