The Effect of Solvent Type on the Infrared Spectrum of Carbon Monoxide Adsorbed Species Selective Gas Chromatographic Detectors

Abstract

The infrared spectrum of Carbon Monoxide adsorbed on a platinum electrode from several solvents was investigated. In N-methylformamide, acetonitrile, and 1,2-dichloroethane, the infrared band attributed to linear bonded CO had experimental Stark tuning rates of 20/cm/V, 22/cm/V, and 19/cm/V, respectively. For each of these solvents, the potential dependence of the band position was found to be linear for the entire potential range investigated. When methanol was the solvent, the plot of the band position versus potential had three distinctly linear portions, each with a different value for the slope. The behavior is explained in terms of the ability of the solvent molecules to closely approach the electrode surface, the polarity of the solvent, and the orientation of solvent molecules with respect to the polarization of the electrode.

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Document Details

Document Type
Technical Report
Publication Date
Jul 15, 1988
Accession Number
ADA200387

Entities

People

  • D. Blackwood
  • M. R. Anderson
  • Stanley Pons

Organizations

  • University of Utah

Tags

Communities of Interest

  • Advanced Electronics
  • Energy and Power Technologies
  • Weapons Technologies

DTIC Thesaurus Topics

  • Abstracts
  • Air Force
  • Carbon Monoxide
  • Chemical Synthesis
  • Chemistry
  • Dielectric Gases
  • Dielectric Permittivity
  • Electrochemical Reactions
  • Electrodes
  • Electromagnetic Fields
  • Frequency
  • Frequency Shift
  • Infrared Spectra
  • Military Research
  • Polarity
  • Spectra
  • Universities

Readers

  • Electrochemical Engineering/ Fuel Cell Technologies
  • Organic Chemistry
  • Spectroscopy.