High Molecular Weight Polyphenylquinoxalines with Increased Solvent Resistance

Abstract

Biphenyl-based bisbenzilmonomers which contain pendant phenylethynyl groups in the 2,2' positions are condensed with 3,3'- diaminobenzidine to make polyphenylquinoxalines (PPQS). Thermal cure of these polymers cause an intramolecular cyclization (TMC) of the phenylethynyl groups to give the rigid 9-phenyldibenzathracene system in the backbone of the polymer. The initial, uncured polymers form tough films which are soluble in m-cresol and chlorinated solvents, but after thermal cure the films become insoluble in all common organic solvents and acids while maintaining their toughness. DSC scans of the cured materials showed small residual exotherms indicating that after vitrification even the intramolecular rotation required for the IMC reaction becomes restricted. Keywords Thermoplastic matrix resins, Solvent resistant thermoplastics.

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Document Details

Document Type
Technical Report
Publication Date
Sep 01, 1988
Accession Number
ADA200997

Entities

People

  • Bruce A. Reinhardt
  • Fred A. Arnold
  • Patricia M. Lindley

Organizations

  • Wright Laboratory

Tags

Communities of Interest

  • Advanced Electronics
  • Air Platforms
  • C4I
  • Energy and Power Technologies

DTIC Thesaurus Topics

  • Aeronautical Laboratories
  • Air Force
  • Air Force Facilities
  • Alcohols
  • Alkanes
  • Chlorides
  • Composite Materials
  • Films
  • Hydroxides
  • Mass Spectra
  • Materials
  • Materials Laboratories
  • Mechanical Properties
  • Polymers
  • Resins
  • Solvents
  • Spectra

Fields of Study

  • Chemistry

Readers

  • Organic Chemistry
  • Polymer Science and Engineering.