Photorefractive Effect in Barium Titanate Crystals

Abstract

Variable-valent iron impurities have been suggested as the source of photorefractive charge carriers in BaTiO3. Very high-purity BaTiO3 crystals were grown with transition-metal impurity levels below the 10 to the 16th power/cc baseline estimate for photorefractivity. Iron-doped crystals also were grown with concentrations of 5, 50, 250, 500, 750, and 1000 ppm Fe. A study of some growth problems effecting purity and perfection of TSSG BaTiO3 crystals was performed. Some preliminary growth experiments in an rf heated Czochralski furnace indicated that it might be possible to utilize the cleaner growth environment of this type of equipment for BaTiO3. Studies were also conducted to investigate the problem of capping after seeding in the TSSG process. It was concluded that convective instabilities in the melt were probably the limiting factor. Keywords: Chemical purification; Crystal growth; Photorefractive effect; Iron doped; Barium titanate.

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Document Details

Document Type
Technical Report
Publication Date
Aug 15, 1988
Accession Number
ADA201406

Entities

People

  • A. Linz
  • H. P. Jenssen

Organizations

  • Massachusetts Institute of Technology

Tags

Communities of Interest

  • Advanced Electronics
  • Energy and Power Technologies
  • Sensors

DTIC Thesaurus Topics

  • Absorption Coefficients
  • Charge Carriers
  • Chemical Synthesis
  • Chemistry
  • Energy Bands
  • Liquids
  • Measurement
  • Military Research
  • Phase Transformations
  • Scattering
  • Spectra
  • Spectroscopy
  • Temperature Gradients
  • Titanium
  • Transition Metals
  • Transition Temperature
  • Wave Mixing

Fields of Study

  • Materials science

Readers

  • Electrochemical Engineering/ Fuel Cell Technologies
  • Optical Physics and Photonics.
  • Semiconductor Device Technology