Examination of Chemical Adsorption and Marine Biofouling on Metal Surfaces Using Raman Scattering Techniques and Electrochemical Impedance Spectroscopy

Abstract

A System has been developed to simulate biofouling of metal surfaces under a range of physical, chemical, and biological conditions. Items of equipment to eliminate and concentrate organic constituents from seawater and to analyze for proteins, glycoproteins, and carbohydrates have been acquired. Teflon fouling chambers have been developed to characterize surface properties of metals in seawater, i.e., adsorption of organic materials, using optical and electrochemical spectroscopic probes. Preliminary studies using these chambers and surface-enhanced Raman spectroscopy demonstrated ability to detect thin layers of pyridine, tryptophan, and phenylalanine adsorbed to silver electrodes. A system to perform waveguide Internal Reflectance Raman Spectroscopy (WIRRS) on thin films adsorbed to a substratum was developed and tested. During preliminary studies, an excellent Raman spectrum was obtained from a 1 micrometer layer of polystyrene. For Electrochemical Impedance Spectroscopy (EIS), electronic hardware was acquired and software was developed to determine the impedance attributes of fouled metal coupons. Preliminary EIS studies using the enzyme, Ribulose Biphosphate Carboxylase, demonstrated the ability to detect adsorption of this protein to a silver electrode.

Open PDF

Document Details

Document Type
Technical Report
Publication Date
Jan 13, 1989
Accession Number
ADA203169

Entities

People

  • Bruce E. Liebert
  • Gordon T. Taylor
  • Howard F. Mower
  • Shiv K. Sharma

Organizations

  • University of HawaiĘ»i System

Tags

Communities of Interest

  • Advanced Electronics

DTIC Thesaurus Topics

  • Amino Acids
  • Carbohydrates
  • Chemical Synthesis
  • Chemistry
  • Dielectric Polymers
  • Electrochemical Cells
  • Materials
  • Organic Materials
  • Photoelectrochemical Cells
  • Raman Scattering
  • Raman Spectra
  • Raman Spectroscopy
  • Spectra
  • Spectroscopy
  • Surface Properties
  • Thin Films
  • Tryptophan

Readers

  • Electrochemical Engineering/ Fuel Cell Technologies
  • Materials Science and Engineering.
  • Nanoscale Plasmonic Nanotechnology

Technology Areas

  • Microelectronics
  • Microelectronics - Graphene