Reactions of Carbon Disulfide and Carbon Dioxide Adducts (eta5-C5H5)(CO) 2Fe-CX2 with Organoiron Electrophiles

Abstract

Availability of analogous pairs of carbon dioxide 1. and carbon disulfide 2. transition-metal complexes permits comparing structure-bonding and chemical reactivity of these ligated heterocumulenes 3. Such comparisons permit us to address the prevalent but questionable attitude that studying the generally more accessible CS2 adducts affords insight into their less stable (or more labile) CO2 congeners 4. We are interested in one pair of bonded heterocumulene complexes, the Fe(CO)2Cp metallodithiocarboxylates Fp-CS2-(NA+, K+) and metallocarboxylates Fp-CO2(Li+,Na+).

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Document Details

Document Type
Technical Report
Publication Date
Oct 03, 1988
Accession Number
ADA203253

Entities

People

  • Alan R. Cutler
  • Bruce E. Landrum
  • John L. Shibley
  • Mary E. Giuseppetti

Organizations

  • Rensselaer Polytechnic Institute

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DTIC Thesaurus Topics

  • Acetonitrile
  • Carbon Dioxide
  • Chemical Reaction Properties
  • Chemical Synthesis
  • Chemistry
  • Column Chromatography
  • Decomposition
  • Electron Transfer
  • Inorganic Carbon Compounds
  • Lewis Acids
  • Materials
  • Metals
  • New York
  • Organic Chemistry
  • Spectra
  • Transition Metals
  • Transitions

Fields of Study

  • Chemistry

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  • Analytical Chemistry
  • Molecular and Cellular Biochemistry
  • Quantum Chemistry