The Glass Transition Temperature as a Parameter for Monitoring the Isothermal Cure of an Amine-Cured Epoxy System

Abstract

The Torsional Braid Analysis (TBA) technique is a convenient one for monitoring the cure of thermosets in terms of the glass transition temperature (Tg) as well as the times to macroscopic gelation and to vitrification. In the process of cure Tg can rise from its initial value (Tgo), through the value corresponding to its molecular gel point (gelTg), to that of the fully cured material (Tg infinity). Differential Scanning Calorimetry (DSC) is also used to measure Tg, and is especially useful in relating Tg to conversion. These techniques have been used to investigate the feasibility of using Tg as the prime parameter for monitoring the complete cure process. The objective is attractive for systems in which there is a one-to-one relationship, independent of the cure temperature, between the Tg of the material and its chemical conversion. It follows for such systems, for example, that the chemical activation energy can be determined equivalently from both the times to reach a fixed conversion and the times to reach a fixed Tg. Keywords: Cure, Vitrification, Glass transition, Kinetics, Time, Temperature, Transformation, Cure diagram, Conversion.

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Document Details

Document Type
Technical Report
Publication Date
Feb 15, 1989
Accession Number
ADA204631

Entities

People

  • G. Wisanrakkit
  • J. K. Gillham

Organizations

  • Princeton University

Tags

Communities of Interest

  • Energy and Power Technologies

DTIC Thesaurus Topics

  • Arrhenius Equation
  • Chemical Engineering
  • Chemical Kinetics
  • Chemistry
  • Critical Temperature
  • Diagrams
  • Engineering
  • Equations
  • Glass Transition Temperature
  • Heat Energy
  • Heat Of Activation
  • Materials
  • Military Research
  • Polymers
  • Transition Temperature
  • Transitions
  • United States

Fields of Study

  • Materials science

Readers

  • Calculus or Mathematical Analysis
  • Materials Science and Engineering.
  • Polymer Science and Engineering.