Fluids, Gels and Glasses Under Extreme Conditions of Pressure and Temperature

Abstract

The NMR and Raman techniques were used to investigate the hydrolysis and condensation mechanism in B2O3-SiO2; A1203-SiO2; and Na2O-Al2O3-SiO2 systems. The solid state NMR techniques were employed together with BET methods to follow the thermal treatment of the gels. In addition to the NMR and Raman techniques, the SANS method was employed to study the effects of fluoride anion catalyst on the sol-gel process involving TMOS. High pressure NMR studies of the dynamic structure of the highly viscous liquids focused on three projects: i) The self-diffusion behavior, and the applicability of hydrodynamic equations at the molecular level for a model lubricant - 2-ethylhexylbenzoate; ii) The effect of the dipole moment on the hydrodynamic behavior of highly polar fluids; iii) The effect of molecular flexibility on the relationship between molecular properties and shear viscosity at extreme conditions of pressure. Boron oxides, Silicon dioxide, Sol gel process, Viscous liquids, Raman, High pressure, Structure property relationship, Aluminum oxide, Sodium oxide.

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Document Details

Document Type
Technical Report
Publication Date
Feb 17, 1989
Accession Number
ADA205292

Entities

People

  • Jiri Jonas

Organizations

  • University of Illinois Urbana–Champaign

Tags

Communities of Interest

  • Advanced Electronics

DTIC Thesaurus Topics

  • Chemical Synthesis
  • Chemistry
  • Crystal Structure
  • Diffraction
  • Dipole Moments
  • Equations
  • Heat Energy
  • Heat Treatment
  • High Pressure
  • Materials
  • Materials Science
  • Measurement
  • Neutron Scattering
  • Scattering
  • Silica Gels
  • Silicon Dioxide
  • Sol Gel Processes

Fields of Study

  • Chemistry

Readers

  • Computational Fluid Dynamics (CFD)
  • Electrochemical Engineering/ Fuel Cell Technologies
  • Polymer Science and Technology