Assignment of the Charge-Transfer Excited States of Bis(N-Heterocyclic) Complexes of Copper(I)

Abstract

Charge-transfer (CT) excited states of metal complexes are provoking intense study, particularly within the context of attempts to design efficient solar energy conversion processes. Since several classes of molecules containing the copper(I) ion have been observed to emit light in fluid solution, attention has been shown to induce electron transfer reactions, complete group theoretic assignments of the nature of the electronic states responsible for the visible absorption and emission spectra have not yet appeared. In this study we focus on the rigid matrix spectra of (Cu(NN)2) species (NN = substituted-2,2'-bipyridine or substituted-1,10-phenanthroline) and propose a group theoretical model to rationalize the results of extensive photophysical measurements on these interesting substances. Synthesis(Chemistry).

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Document Details

Document Type
Technical Report
Publication Date
Mar 21, 1989
Accession Number
ADA206012

Entities

People

  • G. A. Crosby
  • W. L. Parker

Organizations

  • Washington State University

Tags

Communities of Interest

  • Advanced Electronics
  • Energy and Power Technologies
  • Space
  • Weapons Technologies

DTIC Thesaurus Topics

  • Absorption Spectra
  • Chemistry
  • Coordination Complexes
  • Distortion
  • Electron Transfer
  • Electronic States
  • Emission Spectra
  • Energy Levels
  • Geometry
  • Ground State
  • Methanols
  • Military Research
  • Solar Energy
  • Spectra
  • Two Dimensional
  • United States
  • Universities

Fields of Study

  • Chemistry

Readers

  • Materials Science and Engineering.
  • Solar Photovoltaics and Thermoelectric Devices.
  • Theoretical Analysis.

Technology Areas

  • Microelectronics