Exploratory Development on a New Process to Produce Improved RDX crystals: Supercritical Fluid Anti-Solvent Recrystallization

Abstract

Topic A86-142 of the FY 1986 DOD SBIR Solicitation sought investigation of methods which could produce improved intragranular cavity free RDX (cyclotrimethylenetrinitramine) crystals of 100-150 microns size. RDX produced by the current method, recrystallization from cyclohexanone-water solution by evaporative concentration, contains intragranular cavities; they can interfere with the performance of the explosive. Phasex Corporation proposed the use of supercritical fluids as anti-solvents to recrystallize RDX from organic solvent solutions. The concept is based upon the phenomenon of absorption of gas near its critical point by an organic solvent. The absorption of the gas lowers the dissolving power of the organic solvent for RDX resulting in nucleation of RDX. It was suggested that process parameters such as RDX concentration, organic solvent, gas pressure and temperature, rate of introduction of gas and similar factors could be controlled to form the desired particles. Keywords: Explosives, RDX, HMX, Recrystallization, Supercritical fluids, Fine particles. (MJM)

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Document Details

Document Type
Technical Report
Publication Date
May 02, 1988
Accession Number
ADA207760

Entities

People

  • M. P. Coffey
  • P. M. Gallagher
  • V. J. Krukonis

Organizations

  • Ballistic Research Laboratory

Tags

Communities of Interest

  • Energy and Power Technologies
  • Ground and Sea Platforms
  • Weapons Technologies

DTIC Thesaurus Topics

  • Alkanes
  • Alkenes
  • Chemical Synthesis
  • Chemistry
  • Critical Temperature
  • Crystals
  • Cyclohexanones
  • Explosives
  • Fluids
  • Materials
  • Military Research
  • Organic Chemistry
  • Organic Compounds
  • Organic Solvents
  • Particles
  • Phase Diagrams
  • Separators

Fields of Study

  • Chemistry

Readers

  • Agricultural Chemistry/Soil Science
  • Fluid Dynamics.