Radiothermoluminescence Studies of Polymer Solids

Abstract

Radiothermoluminescence (RTL) involves irradiating a sol id at low temperature (77K) with ionizing radiation and observing luminescence when heating the sample at a constant rate (10 K/min). Glow peaks are observed at characteristic temperatures which, for polymers, are diagnostic of the onset of thermally activated molecular motions. A scanning electron microscope (SEM) was modified to irradiate polymer samples with medium energy (5-30 keV) electrons. This SEM-RTL device is more convenient and reliable than other techniques which utilize remote radiation sources though information is confined to the near surface regions of the sample. In particular, the oxygen-free environment of the SEM-RTL experiment permitted observation of high temperature relaxations (up to 150 C or 423 K) for the first time in a number of thermoplastics. Keywords: Polymer relaxation; Molecular motion; Electron irradiation; Charge recombination; Luminescence.

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Document Details

Document Type
Technical Report
Publication Date
Apr 01, 1989
Accession Number
ADA209036

Entities

People

  • Crist Buckley Jr.

Organizations

  • Northwestern University

Tags

Communities of Interest

  • Advanced Electronics
  • Energy and Power Technologies

DTIC Thesaurus Topics

  • Alkenes
  • Chemistry
  • Copolymers
  • Detectors
  • Dielectric Polymers
  • Electron Irradiation
  • Electron Microscopes
  • Energy
  • Energy Transfer
  • Ionizing Radiation
  • Low Temperature
  • Luminescence
  • Optical Properties
  • Polymeric Films
  • Polymers
  • Radiation
  • Scanning Electron Microscopes

Fields of Study

  • Physics

Readers

  • Materials Science and Engineering.
  • Polymer Science and Engineering.
  • Pulsed Power and Plasma Physics.

Technology Areas

  • Microelectronics