A Raman Spectroscopic and Electrochemical Study on Photoinduced Crystal Growth of DABCO (Triethylenediamine) Polyiodide Upon a Silver Electrode

Abstract

Surface Raman spectra of a silver electrode contacting with an acidic solution containing triethylenediamine (DABCO) and sodium iodide showed some new Raman peaks, which were neither the peaks of dissolved DABCO species nor of iodide. These were ascribed to diprotonated DABCO polyiodide crystal, formed and attached onto the laser-irradiated site of the silver electrode. Several facts implied that laser illumination used for the Raman measurement promoted the growth of the crystal; the possibility of photoinduced electrochemical crystal formation was suggested. The mechanisms for this local crystal growth of diprotonated DABCO polyiodide on the silver electrode was examined, as to its dependence upon the solution composition and applied potential. Keywords: Laser-induced crystal growth.

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Document Details

Document Type
Technical Report
Publication Date
Jun 13, 1989
Accession Number
ADA209858

Entities

People

  • D. E. Irish
  • T. Ozeki

Organizations

  • University of Waterloo

Tags

Communities of Interest

  • Weapons Technologies

DTIC Thesaurus Topics

  • Chemistry
  • Crystal Growth
  • Education
  • Engineering
  • Illumination
  • Lasers
  • Light Sources
  • Measurement
  • Metals
  • Military Research
  • Raman Spectra
  • Raman Spectroscopy
  • Security
  • Sodium Compounds
  • Spectra
  • Spectroscopy
  • Universities

Fields of Study

  • Chemistry

Readers

  • Electrochemical Engineering/ Fuel Cell Technologies
  • Electrochemical Surface Science
  • Materials Science and Engineering.

Technology Areas

  • Directed Energy
  • Directed Energy - Pulsed-Laser Deposition