Quenching of N2(a(1IIg), V' = O) by N2, O2, CO, CO2, CH4, H2 and Ar

Abstract

We have determined quenching rate coefficients for N2(a 1 pi(g), V'=O) by Nitrogen Oxygen Hydrogen, CO2, Ar, CH4, and CO using two photon laser excitation. Quenching by N2 appears to proceed via collisional coupling to N2 (a' 1 Sigma U (-), v=O) with a rate coefficient of 2.2 + or - 10 to the -11 power CC3 molecule s. Quenching by Ar is nearly as efficient. Gas-kinetic rate coefficients are obtained for quenching by CO, O2, H2, CO2, and CH4. Collisional energy transfer from N2(a,O) to CO(A) is observed in these experiments. However, quenching by O2, H2, CO2, and CH4 is thought to be reactive. Keywords: Carbon dioxide; Argon; Methane; Carbon monoxide; Lyman Birge; Hopfield bands; Electronic states; Reprints.

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Document Details

Document Type
Technical Report
Publication Date
Feb 15, 1989
Accession Number
ADA210424

Entities

People

  • Byron D. Green
  • William A. Blumberg
  • William J. Kessler
  • William J. Marinelli

Organizations

  • Air Force Research Laboratory

Tags

Communities of Interest

  • Energy and Power Technologies

DTIC Thesaurus Topics

  • Absorption
  • Air Force
  • Data Acquisition
  • Detection
  • Dielectric Gases
  • Dye Lasers
  • Electron Beams
  • Energy
  • Energy Transfer
  • Kinetics
  • Laser Beams
  • Laser Induced Fluorescence
  • Laser Spectroscopy
  • Lasers
  • Measurement
  • Quenching
  • Range Finding

Readers

  • Molecular Photonics/Laser Physics
  • Organic Chemistry
  • Plasma Physics.

Technology Areas

  • Directed Energy
  • Directed Energy - Lasers
  • Microelectronics