Formation of Aluminum Oxide Films from Tris(Hexafluoroacetylacetonato) Aluminum(3) and Tris(Trifluoroacetylacetonato) Aluminumn (3) in the Substrate Temperature Interval 320 C - 480 C in an Argon Ambient Atmosphere

Abstract

The object of the present study was to investigate the thermally activated decompositions of the Al(hfa)3 and Al (tfa)3, varying the decomposition temperature, and examining the chemical composition and electrical properties of the obtained deposits. A study of the thermally activated decomposition of Al(hfa)3 (tris(hexafluoroacetylacetonato)aluminum and Al(tfa)3 (tris(trifluoroacetylacetonato)aluminum) in the gas phase is reported. The decomposition process was carried out in an open tube atmospheric pressure reactor in an inert atmosphere of argon for the substrate temperature interval 320C - 480C. In the case of Al(hfa)3, the chemical vapor deposition process resulted in the deposition of aluminum oxide films while the decomposition of Al(tfa)3 led to the deposition of Al2O3 along with significant quantities of carbon. The breakdown strength of Al/Al2O3/Si capacitors with aluminum oxide films prepared from Al(hfa)3 was found to be higher than 3 MV/cm in most cases. The flat band voltage was positive, indicative of apparent negative oxide charge. Keywords: Thin films, Chemical vapor deposition (CVD), Insulators.

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Document Details

Document Type
Technical Report
Publication Date
Jul 31, 1989
Accession Number
ADA211097

Entities

People

  • Arnold Reisman
  • Dorota Temple

Tags

Communities of Interest

  • Advanced Electronics

DTIC Thesaurus Topics

  • Aluminum Oxides
  • Barometric Pressure
  • Chemical Composition
  • Chemical Engineering
  • Chemical Vapor Deposition
  • Chemistry
  • Electrical Properties
  • Engineering
  • Films
  • Materials
  • Materials Science
  • Military Research
  • Mining Engineering
  • North Carolina
  • Oxide Films
  • Refractive Index
  • Spectra

Readers

  • Electrochemical Engineering/ Fuel Cell Technologies
  • Materials Science and Engineering.
  • Surface Engineering/Surface Coating Technology.

Technology Areas

  • Microelectronics
  • Microelectronics - Graphene