Products of the Hypochlorite Oxidation of Hydrazine Fuels

Abstract

Neutralization of hydrazine fuels with hypochlorite is a recommended procedure for the treatment of fuel spills prior to disposal. Previous research has shown that incomplete reaction of hypochlorite with the methylated hydrazine fuels monomethylhydrazine (MMH) and unsymmetrical dimethylhydrazine (UDMH) leads to a wide variety of byproducts, including N-nitrosoamines, which are believed to be highly carcinogenic. The results presented in this report were obtained as part of a program to assess the environmental implications of using the hypochlorite method for the treatment and disposal of hydrazine fuel spills. The fuels examined were hydrazine, MMH, UDMH, and Aerozine-50. The neutralization products were determined under experimental conditions comparable to those expected for actual spills. The effects of varying the temperature and the pH as well as of aging the final reaction mixture were determined. Quantitative measurements of the nitrosoamines produced are presented. Major and environmentally significant minor products were identified using gas chromatography/mass-spectrometry. Keywords: Chemical reaction. Hydrazine; Monomethylhydrazone (MMH); Unsymmetrical dimethylhydrazine (UDMH).

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Document Details

Document Type
Technical Report
Publication Date
Jun 01, 1989
Accession Number
ADA213557

Entities

People

  • Amrit S. Boparai
  • Jose V. Bonilla
  • Kenneth L. Brubaker

Organizations

  • Argonne National Laboratory

Tags

Communities of Interest

  • Energy and Power Technologies
  • Ground and Sea Platforms

DTIC Thesaurus Topics

  • Aerozine
  • Air Force
  • Carbon Tetrachloride
  • Chemical Reactions
  • Chemical Synthesis
  • Chemistry
  • Engineering
  • Hydrazines
  • Liquid Chromatography
  • Mass Spectra
  • Mass Spectrometry
  • Measurement
  • Organic Chemistry
  • Sodium Compounds
  • Spectra
  • Spectrometry
  • Spectroscopy

Readers

  • Analytical Chemistry
  • Environmental Engineering.
  • Underwater engineering and Marine Technology.