Observation of Atomic Relaxation Near an Interface through Detection of Emitted Fluorescence

Abstract

In this Comment we discuss the general features of spontaneous decay of an atom which is close to the surface of a dielectric (or metal) layer, and this is compared to atomic decay near a four-wave mixing phase conjugator. It is pointed out that the decay or relaxation constants can be expressed entirely in terms of the classical Fresnel coefficients for reflection and transmission of a plane wave, independent of what the explicit forms of these coefficients are. For decay near a dielectric the relaxation constants can be measured directly by counting the number of fluorescent photons per unit of time, after excitation by a laser. For relaxation near a phase conjugator this procedure would require a spectral resolution in the photon detection, since there are two distinct contributions to the fluorescent yield of a two-state atom. The two possible decay mechanisms have different relaxation constants and produce radiation with different frequencies. Atomic relaxation, Near an interface, Emitted fluorescence, Classical fresnel coefficients, Phase conjugator, Four-wave mixing. (jes)

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Document Details

Document Type
Technical Report
Publication Date
Nov 01, 1989
Accession Number
ADA214308

Entities

People

  • Henk F. Arnoldus
  • Thomas F. George

Organizations

  • University at Buffalo

Tags

Communities of Interest

  • Advanced Electronics
  • Air Platforms
  • Weapons Technologies

DTIC Thesaurus Topics

  • Abstracts
  • Air Force
  • Chemical Engineering
  • Chemistry
  • Coefficients
  • Detection
  • Engineering
  • Frequency
  • Materials
  • Materials Science
  • Military Research
  • Molecular Physics
  • New York
  • Physics
  • Plane Waves
  • Radiation
  • Wave Mixing

Fields of Study

  • Physics

Readers

  • Electromagnetic Wave Scattering and Antenna Radiation Engineering
  • Nuclear and Radiation Engineering.
  • Quantum spin resonance or Electron Paramagnetic Resonance spectroscopy.

Technology Areas

  • Directed Energy
  • Directed Energy - Lasers