Preparation and Characterization of Cu2ZnGeS4-ySey
Abstract
Cu2ZnGeS4 can be prepared in both tetragonal stannite and orthorhombic wurtz-stannite phases, whereas Cu2ZnGeSe4 only exists in the tetragonal phase. Selenium can be substituted for sulfur up to 100% in the tetragonal structure of Cu2ZnGeS(4-y)Se(y) prepared at 700 C, and up to 75% in the orthorhombic structure prepared ad 900 C. The temperature at which the phase transformation takes place was found to increase with higher selenium concentration. Iron was substituted into both forms of Cu2Zn(1-x)Fe(x)GeS(4-y) Se(y) and the same in both structures. Keywords: Germanium; Copper; Zinc; Iron; Selenium; Chalcogenides; Optical properties; Semiconducting properties; Non linear optics; Antiferromagnetic interactions.
Document Details
- Document Type
- Technical Report
- Publication Date
- Jan 15, 1990
- Accession Number
- ADA217571
Entities
People
- Aaron Wold
- K. Doverspike
- Kirby Dwight
Organizations
- Brown University