Non-Destructive Characterization of Polymer/Metal Interphases Using Surface-Enhanced Raman Scattering

Abstract

Surface enhanced Raman scattering (SERS) is an analytical technique in which the Raman scattering cross sections of molecules adsorbed onto the roughened surfaces of certain metals are enhanced by as much as six orders of magnitude compared to their value for normal Raman scattering. The mechanisms are associated with the large electric fields that can be induced at the surfaces of metal particles having small radii of curvature and with formation of charge transfer complexes between the adsorbed molecules and the substrate. Enhancement due to the charge transfer mechanism is obtained only for molecules immediately adjacent to the surface but enhancement due to the electromagnetic mechanism may extend several monolayers away from the surface. Since normal Raman scattering by polymers is weak and scattering by molecules adjacent to the substrate is strongly enhanced, SERS can be used for nondestructive characterization of interfaces between polymer films and metals. Silver, Polymers, Materials, Acrylic monomer, Cumene, Hydroperoxide(CHP), Acetylphenylhydrazine(APH), Saccharin, Adhesives, Pyromellitic diimide (PMDI), Surface properties.

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Document Details

Document Type
Technical Report
Publication Date
Jun 01, 1990
Accession Number
ADA222490

Entities

People

  • F. James Boerio
  • Joshua T. Young
  • P. P. Hong
  • W. H. Tsai

Organizations

  • University of Cincinnati

Tags

Communities of Interest

  • Advanced Electronics
  • Air Platforms
  • C4I

DTIC Thesaurus Topics

  • Alkenes
  • Charge Transfer
  • Chemical Synthesis
  • Chemistry
  • Electric Fields
  • Films
  • Geometry
  • Materials
  • Materials Science
  • Molecules
  • Polymeric Films
  • Polymers
  • Raman Scattering
  • Raman Spectroscopy
  • Scattering
  • Spectra
  • Spectroscopy

Readers

  • Atmospheric Science / Meteorology, specifically Wind Wave Turbulence.
  • Nanoscale Plasmonic Nanotechnology
  • Polymer Science and Engineering.