Pyyromethene-BF2 Complexes as Laser Dyes

Abstract

In 1984, less than two decades after its discovery, a review described the dye laser as one of the most useful and practical of tunable coherent sources. Laser dye activity was presumed to reflect a casual relationship with various ancillary properties including photostability, solubility and other interactions with solvent, fluorescence quantum yield, molar extinction of absorption, and minimal overlap of fluorescence with onset of absorption spectral regions, (S-S) and triplet-triplet (T-T). Bathochromic and hyperchromic shifts were introduced by the substitution of auxochromic and antiauxochromic groups but this benefit was often offset by the ability of certain groups, e.g. nitro, cyano, and heavy atoms, to quench laser activity. Since the known dyes were each deficient in one or more properties the search for new structures to offer superior performance standards was undertaken. Keywords: Laser action in pyrromethene-BF2 complex, Synthesis, Boron trifluoride, TMP, PMP, HMP, PMDEP, Chlorosulfonation, PMPDS, Condensation.

Open PDF

Document Details

Document Type
Technical Report
Publication Date
May 24, 1990
Accession Number
ADA223562

Entities

People

  • Joseph H. Boyer
  • Kannappan Thangaraj
  • Lionel T. Wolford
  • Mayur Shah
  • Mou-ling Soong

Tags

Communities of Interest

  • Biomedical
  • Energy and Power Technologies
  • Weapons Technologies

DTIC Thesaurus Topics

  • Alcohols
  • Alkanes
  • Chemical Synthesis
  • Chemistry
  • Dye Lasers
  • Laser Dyes
  • Lasers
  • Military Research
  • Organic Chemistry
  • Quantum Yields

Readers

  • Chemistry (specifically Chemical Fluorescence)
  • Organic Chemistry
  • Systems Analysis and Design

Technology Areas

  • Directed Energy
  • Directed Energy - Lasers
  • Quantum Computing