Catalytic Agent Degradation on Oxide Films and in Microheterogeneous Solution Systems

Abstract

Both photocatalytic and dark decompositions of the organophosphate compounds diethylbenzylphosphonate (DBP) and diethylethylphosphonate (DEP) were investigated in the presence of hydrogen peroxide as oxidant. The role of colloidal TiO2 and ferric sulfate as promoters for the complete mineralisation of the agent was explored. Fundamental studies under the same experimental conditions on the degradation of the aromatic species nitro-o-oxylene (NOX) were likewise undertaken in order to more clearly elucidate the aromatic ring breaking mechanism. The combined effects of dark catalysis and band gap excitation were investigated.

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Document Details

Document Type
Technical Report
Publication Date
Jun 20, 1990
Accession Number
ADA224199

Entities

People

  • Michael Grätzel

Tags

Communities of Interest

  • Materials and Manufacturing Processes

DTIC Thesaurus Topics

  • Absorption
  • Absorption Spectra
  • Aqueous Solutions
  • Band Gaps
  • Charge Carriers
  • Chemical Synthesis
  • Chemistry
  • Decomposition
  • Degradation
  • Energy Bands
  • Hydrogen
  • Organophosphates
  • Oxidation
  • Oxide Films
  • Oxides
  • Reaction Time
  • Rocket Oxidizers

Readers

  • Analytical Chemistry
  • Electrochemical Engineering/ Fuel Cell Technologies
  • Quantum spin resonance or Electron Paramagnetic Resonance spectroscopy.