FTIR Studies Reveal That Silicon-Containing Laser-Induced Desorption Products Are Surface Reaction Intermediates

Abstract

Silicon containing laser induced desorption (LID) products such as SiOH and SiNH2 have been observed from Si(111)7x7 surfaces exposed to H2O and NH3. Assuming that the LID species were derived from surface reaction intermediates, these LID products were employed to examine the thermal stability of the SiOH and SiNh2 surface species. Fourier transform infrared (FTIR) transmission spectroscopy was recently utilized to monitor the decomposition of SiOHand siNH2 surface species following the dissociative adsorption of H2O and HH3 on porous silicon surfaces. The FTIR results on porous silicon surfaces were in excellent agreement with the previous LID studies on Si(111)7x7. The correspondence between the FTIR and LID investigations indicated that silicon- containing LID products are derived from silicon surface reaction intermediates.

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Document Details

Document Type
Technical Report
Publication Date
Jul 31, 1990
Accession Number
ADA226582

Entities

People

  • A. C. Dillon
  • P. A. Coon
  • Paridhi Gupta
  • S. M. George

Organizations

  • Stanford University

Tags

DTIC Thesaurus Topics

  • Auger Electron Spectroscopy
  • Auger Electrons
  • California
  • Chemical Reactions
  • Chemistry
  • Classification
  • Decomposition
  • Desorption
  • Infrared Spectra
  • Military Research
  • Security
  • Spectra
  • Spectroscopy
  • Surface Chemistry
  • Surface Reactions
  • Thermal Stability
  • United States

Readers

  • Electrochemical Engineering/ Fuel Cell Technologies

Technology Areas

  • Directed Energy