Chemical Characterization of Simulated Boiling Water Reactor Coolant

Abstract

An in-pile facility is being constructed at MIT to simulate the thermal-hydraulic, radiation, and coolant-chemistry environment of a Boiling Water Reactor (BWR). The primary purpose of this BWR Coolant Chemistry Loop (BCCL) is to characterize coolant radiolysis chemistry by measurement of O2, H2O2, H2, electrode potential, pH, etc.. However, hydrogen peroxide, which is highly oxidizing, readily decomposes on system surfaces. Therefore, the measurement of, and computer code prediction of, the concentration of H2O2 in the BCCL emerges as the primary challenge to achieving the BCCL project objectives. The principal objective of this work was to design, build and test a coolant sampling system capable of measuring H2O2 to support BCCL operation. This included the requirement to investigate high-temperature H2O2 behavior sufficiently, both analytically and experimentally, to develop the design objectives for the sampling system. The high-temperature experiments on H2O2 behavior showed that surface decomposition was the same for the materials tested - titanium, aluminum and stainless steel, and minimal decomposition of H2O2 occurred when the sample line tubing wall was cooled. (JES)

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Document Details

Document Type
Technical Report
Publication Date
May 01, 1990
Accession Number
ADA226654

Entities

People

  • Verrdon H. Mason

Organizations

  • Massachusetts Institute of Technology

Tags

Communities of Interest

  • Energy and Power Technologies
  • Ground and Sea Platforms
  • Human Systems

DTIC Thesaurus Topics

  • Chemical Engineering
  • Chemical Kinetics
  • Chemical Reaction Properties
  • Chemical Reactions
  • Chemical Synthesis
  • Chemistry
  • Computational Fluid Dynamics
  • Computers
  • Construction
  • Decomposition
  • Fluid Dynamics
  • Materials
  • Materials Science
  • Measurement
  • Nuclear Power Plants
  • Nuclear Reactors
  • Steady State

Fields of Study

  • Physics

Readers

  • Combustion and Flow Dynamics.
  • Computational Modeling and Simulation
  • Organic Chemistry