Observation of Spectral Diffusion in Crystals Using Single Impurity Molecules

Abstract

Early measurements of the optical absorption spectrum of a single impurity molecule in a solid at low temperatures, while intriguing, nevertheless produced insufficient signal-to-noise ratio for the observation of new physical effects. Recent advances in high-efficiency fluorescence excitation spectroscopy have removed this obstacle. For the case of pentacene molecules inp-terphenyl, both stable as well as spectrally diffusing single molecules can be observed.

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Document Details

Document Type
Technical Report
Publication Date
Oct 31, 1990
Accession Number
ADA231338

Entities

People

  • W. E. Moerner
  • W. P. Ambrose

Organizations

  • International Business Machines Corporation (Armonk, NY)

Tags

Communities of Interest

  • Materials and Manufacturing Processes
  • Weapons Technologies

DTIC Thesaurus Topics

  • Absorption
  • Absorption Spectra
  • Chemistry
  • Classification
  • Crystals
  • Detuning
  • Dye Lasers
  • Frequency
  • Laser Beams
  • Lasers
  • Low Temperature
  • Military Research
  • Optical Absorption
  • Spectra
  • Spectroscopy
  • Time Dependence
  • United States

Fields of Study

  • Physics

Readers

  • Materials Science and Engineering.
  • Molecular Photonics/Laser Physics
  • Systems Analysis and Design