Effects of Abasic Sites on Triple Helix Formation Characterized by Affinity Cleaving

Abstract

The stability of triple helical complexes between oligodeoxyribonucleotides containing one or two abasic 1,2-dideoxy-D-ribose residues bound to single 15-17 base pair sites within short duplex (30mer) or plasmid DNA (4.9 kbp) was examined by affinity cleaving. The triplets are significantly less stable than triplexes having the matched counterparts, T AT, C+GC and G TA. Oligodeoxyribonucleotide-directed triple-helix formation offers a chemical approach for the sequence-specific binding of double-helical DNA that is 10 to the 6th power times more specific than restriction enzymes. Because triple-helix formation by pyrimidine oligodeoxyribonucleotides is limited to mostly purine tracts (T AT, C+GC triplets), it is desirable to find a general solution whereby oligodeoxyribonucleotides (or other analogs) could be used to bind all four base pairs of intact duplex DNA.

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Document Details

Document Type
Technical Report
Publication Date
Jun 01, 1991
Accession Number
ADA237528

Entities

People

  • D. A. Horne
  • P. B. Dervan

Organizations

  • California Institute of Technology

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DTIC Thesaurus Topics

  • Acetic Acid
  • Alcohols
  • Chemical Engineering
  • Chemical Synthesis
  • Chemistry
  • Electrophoresis
  • Gel Electrophoresis
  • Military Research
  • Organic Chemistry
  • Procurement
  • Pyrimidines
  • Security
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  • Standards
  • Thymidines
  • United States
  • United States Government

Fields of Study

  • Biology
  • Chemistry

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  • Molecular Genetics