Thermochemistry of Hydrocarbon Decomposition and Relationship to Properties of PECVD Diamond Films

Abstract

Considerable empirical research has been performed in the field of diamond film growth over the past fifteen years. However, this approach has proven insufficient in optimizing the deposition process. Also, no deposition mechanism has become universally accepted. A combination of in situ plasma diagnostic instruments, diamond film characterization, and computer modeling has been used to produce a self-consistent model of diamond-producing DC plasmas and to optimize the deposition process in terms of bonding type (i.e., graphite vs. diamond) and growth rate. The effects of important deposition parameters including methane concentration in hydrogen, current, electrode spacing, and pressure on both film and plasma characteristics have been analyzed. The presence of a negative electric field at the anode (or substrate electrode) has been determined to be necessary for the growth of high quality diamond films. The magnitude of this field is strongly dependent on pressure. Control of this field will be possible by monitoring with a Langmuir probe and controlling pressure, leading to in situ process control.

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Document Details

Document Type
Technical Report
Publication Date
Mar 31, 1991
Accession Number
ADA237793

Entities

People

  • Linda S. Plano

Tags

Communities of Interest

  • Energy and Power Technologies

DTIC Thesaurus Topics

  • Charged Particles
  • Chemical Analysis
  • Chemical Vapor Deposition
  • Chemistry
  • Dissociation
  • Electrons
  • Graphitic Materials
  • Mass Spectrometers
  • Mass Spectrometry
  • Materials
  • Materials Processing
  • Materials Science
  • Measurement
  • Spectra
  • Spectrometers
  • Spectrometry
  • Spectroscopy

Readers

  • Combustion science or combustion engineering.
  • Theoretical Analysis.
  • Thin Film Deposition Science.

Technology Areas

  • Space
  • Space - Hall-Effect Thruster