Studies on Macromolecules Derived from Polypyrazolylboron and Related Boron-Nitrogen Species

Abstract

Studies on the synthesis, characterization, and chemical behavior of pyrazaboles, semi-pyrazaboles, poly(1-pyrazolyl)borates, boroxins, diboroxanes, and borazines have been performed. Several pathways for the synthesis and chemical modification of pyrazaboles, which are characterized by the general framework and contain a central B2N4 heterocycle, have been developed. Besides normal pyrazaboles triply bridged derivatives with repeating and semi- pyrazaboles have been prepared and characterized, including a series of X-ray crystal structure determinations. Various polynuclear materials containing boron units (M=metal) and poly(1-pyrazolyl)borates have also been studied. Some corresponding derivatives of azoles other than pyrazole have been investigated highlighted by the preparation and characterization of a novel porphine analogue containing a B4N12 heterocycle.

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Document Details

Document Type
Technical Report
Publication Date
Oct 01, 1991
Accession Number
ADA242588

Entities

People

  • Kurt Niedenzu

Organizations

  • University of Kentucky

Tags

Communities of Interest

  • C4I

DTIC Thesaurus Topics

  • Alkali Metals
  • Analogs
  • Chemistry
  • Crystal Structure
  • Crystals
  • Kentucky
  • Macromolecules
  • Materials
  • Metals
  • Military Research
  • Nitrogen
  • Nitrogen Compounds
  • Pyrazoles
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Fields of Study

  • Chemistry

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  • Organic Chemistry