Cationic Bulk Polymerization of Vinyl Ethers in the Liquid Crystalline Phase

Abstract

Cationic bulk polymerization of liquid crystalline phenyl benzoate and biphenyl vinyl ethers was performed using either thermal or photochemical initiation by onium salts. High molecular mass polymers having narrow molecular mass distribution were produced in high yields at very high temperature. Seemingly, the polymerization system could stabilize the growing species and thus reduce the amount of chain transfer reactions. Thin films of the monomers were oriented in their liquid crystalline state by the use of conventional ordering techniques used for low molar mass liquid crystals. On subsequent polymerization the orientation was preserved giving liquid crystalline thin films having a very high degree of order.

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Document Details

Document Type
Technical Report
Publication Date
Oct 30, 1991
Accession Number
ADA242627

Entities

People

  • A. Hult
  • A. Percec
  • H. Jónsson
  • U. W. Gedde

Organizations

  • Case Western Reserve University

Tags

Communities of Interest

  • Advanced Electronics

DTIC Thesaurus Topics

  • Alkenes
  • Chemical Shifts
  • Classification
  • Films
  • High Temperature
  • Macromolecules
  • Military Research
  • Oligomers
  • Phase
  • Phase Transformations
  • Polymeric Films
  • Polymers
  • Security
  • Spectra
  • Thick Films
  • Thin Films
  • Universities

Fields of Study

  • Chemistry

Readers

  • Organic Chemistry
  • Thin Film Deposition Science.