Molecular Composites from Rod and FlexiblePolyquinolines

Abstract

The properties of blends of two polyquinolines and block copolymers of the same polymers have been studied as the basis for a molecular composite. The polyquinolines differ only in the presence or absence of an oxygen atom in the chain backbone. The chain conformation is found to be extended, with a persistence length of 20 nm without the oxygen linkage. The chain adopts a flexible conformation when the oxygen is present. Both forms, and their copolymer, were synthesized in this study. The results show that although the thermodynamically expected phase separation can be partially frustrated in the preparation of blends of the two polymers, the enhanced mobility at the elevated temperatures needed for processing the solid blend leads to substantial phase separation, with consequent deterioration of mechanical properties.

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Document Details

Document Type
Technical Report
Publication Date
Nov 01, 1991
Accession Number
ADA243634

Entities

People

  • D. R. Uhlmann
  • Elliot R Bernstein
  • G. C. Berry
  • J. K. Stille

Organizations

  • Colorado State University

Tags

Communities of Interest

  • Air Platforms
  • C4I
  • Energy and Power Technologies

DTIC Thesaurus Topics

  • Block Copolymers
  • Composite Materials
  • Copolymers
  • Diffraction
  • Electron Microscopy
  • Films
  • Light Scattering
  • Materials
  • Materials Laboratories
  • Materials Science
  • Mechanical Properties
  • Molecules
  • Neutron Scattering
  • Phase Separation
  • Polymeric Films
  • Polymers
  • Scattering

Fields of Study

  • Chemistry
  • Materials science

Readers

  • Polymer Science and Technology

Technology Areas

  • Microelectronics