Optical Spectra and Kinetics of Single Impurity Molecules in a Polymer: Spectral Diffusion and Persistent Spectral Hole-Burning

Abstract

Using high efficiency fluorescence excitation techniques, optical spectra of single impurity molecules of perylene in a poly(ethylene) matrix can be obtained at 1.5 K. Analysis of such spectra show a variety of spectral diffusion effects, including fast resonance frequency changes on the 1-100 MHz scale which lead to a range of apparent linewidths, as well as discontinuous jumps in the resonance frequency of 10-1000 MHz on a longer time scale. In addition, light induced changes in resonance frequency of a single molecule (persistent spectral hole-burning) have been conclusively observed by showing that the burning time decreases with increasing laser power. Surprisingly, hole- burned single molecule often spontaneously return to the original frequency in 1-100 s. Measurements of the burning time for a large number of hole-burning events for the same simple molecule yield an exponential burn time distribution, which is the first direct measurement to our knowledge for the stochastic kinetics of a single molecule.

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Document Details

Document Type
Technical Report
Publication Date
Nov 07, 1991
Accession Number
ADA243749

Entities

People

  • T. Basche
  • W. E. Moerner
  • W. P. Ambrose

Organizations

  • International Business Machines Corporation (Armonk, NY)

Tags

Communities of Interest

  • Energy and Power Technologies

DTIC Thesaurus Topics

  • Amorphous Materials
  • Amplitude
  • Chemistry
  • Classification
  • Combustion
  • Detection
  • Frequency
  • Intervals
  • Kinetics
  • Laser Beams
  • Laser Spots
  • Lasers
  • Military Research
  • Quantum Efficiency
  • Quantum Yields
  • Spectroscopy
  • Time Intervals

Fields of Study

  • Physics

Readers

  • Mathematics or Statistics
  • Optical Physics and Photonics.
  • Quantum spin resonance or Electron Paramagnetic Resonance spectroscopy.

Technology Areas

  • Directed Energy
  • Directed Energy - Lasers