Improved Method for Synthesis of Difunctional Fluoroalcohols.

Abstract

A series of fluorinated diacids were prepared by the direct fluorination of hydrocarbon acid derivitives with fluorine gas. These diacids were then reduced to fluorinated alcohols with sodium borohydride. A miniplant capable of producing fluorinated diols at a rate of five pounds per day was constructed to demonstrate the technology. The resulting diols wer obtained in much better yields than by conventional synthetic fluorocarbon chemistry. In addition, diols of perfluoropolyether acids were made that are not available using other synthetic methods. The compounds prepared for this contract were 2, 2,3,3,4,4-hexafluoropentane-1,5-diol, 2,2,3,3,4,4,5,5-octofluorohexane-1,6-diol, 2,2,4,4,5,5,7,7-octofluoro-3,6-dioxaoctane-1,8-diol, and 2,2,3,3,4,4,6,6,7,7,8, 8,9,9,11,11,12,12,13,13,14,14,16,16,17,17,18,18-octacosafluoro-5,10,15- trioxanonadecane-1,19-diol.

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Document Details

Document Type
Technical Report
Publication Date
Jun 03, 1991
Accession Number
ADA245070

Entities

People

  • Hajimu Kawa
  • Richard J. Lagow
  • Thomas R. Bierschenk
  • Timothy J. Juhlke

Tags

Communities of Interest

  • Human Systems
  • Sensors
  • Weapons Technologies

DTIC Thesaurus Topics

  • Alcohols
  • Aluminum Oxides
  • Chemical Synthesis
  • Chemistry
  • Fluorination
  • Fluorine
  • Fluoropolymers
  • Hydrocarbons
  • Materials Laboratories
  • Materials Processing
  • Materials Science
  • Military Research
  • Organic Chemistry
  • Organic Compounds
  • Polyethylene Glycols
  • Polymer Chemistry
  • Resins

Fields of Study

  • Chemistry

Readers

  • Organic Chemistry