Chemically Sensitive Microelectrochemical Devices: New Approaches to Sensors

Abstract

Described herein are the proof of concept results demonstrating a new approach to electrochemical sensors based upon chemically sensitive microelectrochemical devices. A typical device consists of at least two individually addressable electrodes. The working electrode is a microelectrode and is derivatized with at least one molecule that has a chemically sensitive formal potential and serves as the indicator, and one molecule that has a chemically insensitive formal potential and serves as a reference. The indicator and reference molecules are confined to the electrodes either by monolayer self assembly techniques or by dissolving in a thin film of solid electrolyte. Detection in these systems is accomplished by measuring either the potential difference associated with current peaks for oxidation (or reduction) of microelectrode confined redox reagents.

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Document Details

Document Type
Technical Report
Publication Date
Feb 04, 1992
Accession Number
ADA245798

Entities

People

  • C. A. Mirkin
  • D. Ofer
  • J. J. Hickman
  • J. R. Valentine
  • M. S. Wrighton

Organizations

  • Massachusetts Institute of Technology

Tags

Communities of Interest

  • Advanced Electronics
  • Sensors
  • Weapons Technologies

DTIC Thesaurus Topics

  • Carbon Monoxide Indicators
  • Chemical Synthesis
  • Chemistry
  • Detection
  • Detectors
  • Electrochemistry
  • Films
  • Military Research
  • Mixtures
  • Monomolecular Films
  • Photoelectrochemical Cells
  • Self Assembly
  • Spectra
  • Spectrometers
  • Thin Films
  • United States
  • Voltammetry

Fields of Study

  • Chemistry

Readers

  • Electrochemical Engineering/ Fuel Cell Technologies