Genetic Engineering of a Type II DHFR

Abstract

Three areas of research on the Type 11 DHFR have been pursued. These were (1) analysis of structure and mechanism of the enzyme; (2) stability effects on the protein and variants in vivo and in vitro; and (3) plasmid constructs of mutants and expression of mutants. Studies of the first have shown that the stereochemistry of hydride transfer from NADPH to dihydrofolate placed this enzyme as one of the A-stereospecific class of dehydrogenases. The interaction of the enzyme with cofactors has been studied by equilibrium dialysis, proton NMR spectroscopy and differential scanning calorimetry. Two types of complexes have been found, and a shift of conformation between 5.0 and 5.9 was observed. In the mutant work, several mutants in the proposed active site have been formed. Some were inactive in vivo. In certain cases (e.g., Glu 58 yields Gin 58) the enzyme was rather unstable to protease attack in vivo. This factor was even more pronounced in sup+ strains.

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Document Details

Document Type
Technical Report
Publication Date
Jul 01, 1991
Accession Number
ADA246099

Entities

People

  • G. N. Bennett

Organizations

  • Rice University

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DTIC Thesaurus Topics

  • Albumins
  • Biochemistry
  • Biology
  • Biomedical And Dental Materials
  • Cell Biology
  • Cellular Structures
  • Chemical Analysis
  • Chemical Shifts
  • Chemistry
  • Enzyme Inhibitors
  • Escherichia Coli
  • Gel Electrophoresis
  • Genetic Engineering
  • Liquid Chromatography
  • Materials
  • Molecular Biology
  • Recombinant Proteins

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  • Chemistry

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  • Molecular Genetics
  • Molecular and Cellular Biochemistry

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  • Biotechnology
  • Biotechnology - Cancer Biotech