Toluene-Ammonia Cluster: Ion Fragmentation and Chemistry

Abstract

The Toluene ammonia cluster system is studied by mass resolved excitation spectroscopy: like the toluene water system, an extensive ion chemistry is found to exist generating ammonia solvated protons and (solvated) benzyl radicals. Extensive cluster fragmentation is observed even at threshold ionization energies. Nozzle deuteration studies are applied to elucidate the extensive ion chemistry of this cluster system. Proton transfer cluster fragmentation reactions in this system are assisted by solvation of the benzyl radical or toluene ion: cluster fragmentation by loss of a single ammonia molecule is not observed. Fragmentation is so extensive for this system that spectra could not be identified with parent clusters.

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Document Details

Document Type
Technical Report
Publication Date
Feb 04, 1992
Accession Number
ADA246253

Entities

People

  • Elliot R. Bernstein
  • Shengxi Li

Organizations

  • Colorado State University

Tags

Communities of Interest

  • Energy and Power Technologies

DTIC Thesaurus Topics

  • Abstracts
  • Chemical Reactions
  • Chemistry
  • Classification
  • Colorado
  • Contracts
  • Elements
  • Exchange Reactions
  • Governments
  • Identification
  • Intensity
  • Ionization
  • Military Research
  • Nitrogen Compounds
  • Security
  • Spectra
  • Spectroscopy

Fields of Study

  • Chemistry

Readers

  • Combustion science or combustion engineering.
  • Quantum Chemistry