Effect of Lead Oxide and Titania on the Structure, Morphology and Superconductivity of Y-Ba-Cu-O Ceramic Materials
Abstract
The effect of the addition of PbO and TiO2, in the concentration range 0 15 wt.%, on crystal structure, morphology and superconductivity of YBa2CU306+X was investigated. The results suggest that the addition of either TiO2 or PbO (for PbO concentration above 3 wt.%) reduces the primary particle size of YBa2CU306+X. Both TiO2 and PbO tends to stabilize the non superconducting tetragonal phase at the expense of superconducting orthorhombic phase of YBa2CU306+X. The orthorhombic - tetragonal phase transformation appears to be related to the additive induced oxygen depletion of YBa2CU306+X to form Y2BaCuOy. Such a phase transformation-process not only increases the normal state resistance of the superconductor, but also lowers the superconducting transition temperature.
Document Details
- Document Type
- Technical Report
- Publication Date
- Jan 31, 1992
- Accession Number
- ADA248706
Entities
People
- A. S. Rao
Organizations
- Naval Surface Warfare Center Carderock Division