Time-resolved Two-laser Probe of Cr(CO)6 Photodissociation Dynamics

Abstract

We have examined the photodissociation of jet-cooled Cr(CO)6 using a time-resolved, two-laser multiphoton dissociation (MPD) technique with fluorescence detection of the atomic photofragments. We have observed that the rate of appearance of Cr(CO)4 via 248-nm photolysis of Cr(CO)6 is slower if the Cr(CO)6 has first been cooled in a supersonic expansion. We suggest the difference in the observed rates is due to slower intersystem crossing in the transient Cr(CO)5 following impulsive loss of the first CO ligand from the jet- cooled hexacarbonyl. This intersystem crossing is thought to be facilitated by low-energy OC-Cr-CO bending modes, which are probably not accessible by one- photon absorption from the ground state Cr(CO)6. We discuss the utility of our time-resolved MPD/atomic fluorescence technique as a general dynamical probe for metal carbonyl photodissociation.

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Document Details

Document Type
Technical Report
Publication Date
Jun 01, 1992
Accession Number
ADA250930

Entities

People

  • James F. Garvey
  • Robert Deleon
  • William R. Peifer

Organizations

  • University at Buffalo

Tags

Communities of Interest

  • Energy and Power Technologies

DTIC Thesaurus Topics

  • Absorption
  • Abstracts
  • Carbonyl Complexes
  • Chemical Reactions
  • Chemistry
  • Crossings
  • Dissociation
  • Electronic States
  • Fluorescence
  • Ground State
  • Laser Pulses
  • Lasers
  • Molecular Beams
  • New York
  • Photodissociation
  • Photolysis
  • Physical Chemistry

Fields of Study

  • Physics

Readers

  • Molecular Photonics/Laser Physics
  • Neurological Diseases/Conditions/Disorders

Technology Areas

  • Directed Energy
  • Directed Energy - Lasers
  • Hypersonics
  • Hypersonics - Hypersonic Flight