Design and Synthesis of Molecular Systems Capable of Supporting Intracavity Chemical Reactions

Abstract

This project involves the synthesis of molecules containing concave functional groups capable of supporting chemical reactions. Salient sub-problems have to do with the distinction between steric encumbrance and steric hindrance, and with development of well documented intracavity covalent bond-forming reactions. Host molecules bearing functional groups capable of hydrogen bond formation, metal ion complexation, and aldimine condensation are of primary interest, their functional groups being in a sterically encumbered but not hindered environment. The structural motif involves construction of cyclophanes bearing the desired reactive group oriented in an inward-pointing manner, in combination (optionally) with structural features that enhance binding of the external co-reactor.

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Document Details

Document Type
Technical Report
Publication Date
May 13, 1992
Accession Number
ADA251024

Entities

People

  • Howard W. Whitlock Jr

Tags

DTIC Thesaurus Topics

  • Chemical Reactions
  • Chemical Synthesis
  • Chemistry
  • Coordination Complexes
  • Covalent Bonds
  • Design Criteria
  • Hydrogen
  • Hydrogen Bonds
  • Imines
  • Military Research
  • Molecules
  • Oxides
  • Phosphine
  • Phosphine Oxides
  • United States
  • United States Government

Fields of Study

  • Chemistry

Readers

  • Molecular and Cellular Biochemistry
  • Optical Physics and Photonics.
  • Organic Chemistry