Adsorption and Accommodation of Xe on Pt(111)

Abstract

We have recorded real-space images of Xe adatoms on the Pt(III) surface using a scanning tunneling microscope. In the dilute coverage limit, we find nearly all the Xe atoms at step edges. From this observation we deduce a lower limit of hundreds of Angstroms that Xe atoms scatter across the surface upon adsorption. This result is in sharp contrast to previous studies of metal atom adsorption on metal surfaces in which it is believed that a large fraction of the impinging atoms remain at their point of impact at low surface temperature. For Xe, once the step sites are nearly saturated, point defects on the Pt(III) surface nucleate the growth of compact, incommensurate, rotationally ordered Xe islands. Thus, we have imaged the initiation of the growth of a surface overlayer, and have identified the sites at which this growth begins.

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Document Details

Document Type
Technical Report
Publication Date
May 25, 1992
Accession Number
ADA251661

Entities

People

  • D. M. Eigler
  • Paul S. Weiss

Organizations

  • Pennsylvania State University

Tags

Communities of Interest

  • Energy and Power Technologies

DTIC Thesaurus Topics

  • Adsorption
  • Base Pressure
  • Chambers
  • Chemistry
  • Crystal Lattices
  • Crystals
  • Diffraction
  • Diffusion
  • Energy
  • Kinetic Energy
  • Low Temperature
  • Measurement
  • Military Research
  • Point Defects
  • Quartz Crystal Microbalances
  • Scattering
  • Surface Temperature

Fields of Study

  • Physics

Readers

  • Electrochemical Engineering/ Fuel Cell Technologies
  • Materials Science and Engineering.
  • Molecular Photonics/Laser Physics

Technology Areas

  • Space
  • Space - Hall-Effect Thruster