Differentiation among Isomeric Polyfunctional Nitroaromatics by Dimethyl Ether Chemical Ionization Mass Spectrometry in a Conventional Ion Source

Abstract

Since aromatic positional isomers frequently cannot be reliably distinguished by their electron ionization (EI) or chemical ionization (CI) mass spectra, interest in new selective CI reagents has been widespread. Among the most recent and promising were nitric oxide using a Townsend discharge technique and dimethyl ether (DME) in a quadrupole ion trap mass spectrometer (ITMS). For a number of difunctional oxyaromatics in the ITMS, the adduct ions resulting from ion-molecule reactions with reagent-derived ions demonstrated both functional group and positional selectivity, whereas in a conventional ion source no structural selectivity was observed. The adduct ions observed were M + 1+, M + 13 +, M + 15 +, M + 45 + and M + 47 + (proton, methine, methyl, methoxymethylene and protonated DME adducts).

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Document Details

Document Type
Technical Report
Publication Date
Jan 01, 1992
Accession Number
ADA252815

Entities

Organizations

  • United States Army Biological Warfare Laboratories

Tags

Communities of Interest

  • Biomedical

DTIC Thesaurus Topics

  • Biomedical Research
  • Diesel Fuels
  • Ion Sources
  • Ion Traps
  • Ionization
  • Ions
  • Mass Spectra
  • Mass Spectrometers
  • Mass Spectrometry
  • Spectra
  • Spectrometers
  • Spectrometry
  • Tnt

Fields of Study

  • Chemistry

Readers

  • Molecular Photonics/Laser Physics
  • Organic Chemistry

Technology Areas

  • Microelectronics