Air and Water Stable 1-Ethyl-3-methylimidazolium Based Ionic Liquids

Abstract

A series of novel air and water stable low melting salts based upon the 1-ethyl-3-methylimidazolium cation (EtMeim+) have been prepared and characterized; two salts, (EtMeim)BF4 and (EtMeim)MeCO2, are liquids under ambient conditions. Alkylpyridinium (Pry+) chloroaluminate based ambient temperature ionic liquids have been known since the 1950s, however, it was the discovery of EtMeim+ based chloroaluminate ionic liquids in 1982 that afforded the impetus for a dramatic increase in activity in the area. The latter class of compounds exhibits a wider liquidus range and an electrochemical window of >3.0 V and has therefore become of great interest from both an electrochemical and a synthetic perspective. A considerable drawback of ambient ionic liquids concerns the need to protect rigorously the ionic liquids from moisture and other oxide impurities and the tendency of many substrates to react with halometallates.

Open PDF

Document Details

Document Type
Technical Report
Publication Date
Jan 01, 1992
Accession Number
ADA255787

Entities

People

  • John S. Wilkes
  • Michael J. Zaworotko

Organizations

  • Air Force Research Laboratory

Tags

Communities of Interest

  • Air Platforms

DTIC Thesaurus Topics

  • Air Force
  • Chemical Compounds
  • Chemistry
  • Crystal Structure
  • Crystals
  • Hydrogen
  • Hydrogen Bonds
  • Ionic Liquids
  • Ions
  • Liquids
  • Materials
  • Materials Science
  • Melting
  • Melting Point
  • New York
  • Physical Properties
  • United States

Fields of Study

  • Chemistry

Readers

  • Materials Science and Engineering.
  • Organic Chemistry
  • Systems Analysis and Design