Characterization of Vesicle and Microemulsion Microstructures

Abstract

We have determined micellar aggregation numbers for a number of single- and double-chain surfactants using time-resolved fluorescence quenching and small angle neutron scattering as functions of surfactant concentration, chain length and temperature. The force between dialkyldimethylammonium bromide and acetate bilayers was measured with the surface forces apparatus as a function of added salt and temperature. Using atomic force microscopy we obtained images of normal and interdigitated bilayers. We identified a new mechanism for emulsification in which a W/O microemulsion inverts to a O/W macroemulsion upon contact with water. We characterized high internal phase emulsions and related their structures to the HLB temperature of the surfactant. We prepared the first reversed vesicles containing water shells separated by well-defined hydrocarbon interior and exterior phases. We demonstrated how both normal and reversed micelles can be prepared from the same oil/water/surfactant system near the HLB temperatures of the surfactant by simply varying the concentration of components. Self-Assembly, Amphiphiles, Reversed Vesicles, Surface Forces Apparatus, Atomic Force Microscopy, High Internal Volume Phase Emulsions.

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Document Details

Document Type
Technical Report
Publication Date
Sep 01, 1992
Accession Number
ADA257036

Entities

People

  • D. F. Evans

Organizations

  • University of Minnesota

Tags

Communities of Interest

  • Air Platforms
  • Energy and Power Technologies
  • Human Systems

DTIC Thesaurus Topics

  • Alkanes
  • Dielectric Polymers
  • Dispersions
  • Electron Microscopy
  • Emulsions
  • Failure Mode And Effect Analysis
  • Hydrocarbons
  • Liquid Crystals
  • Measurement
  • Mechanical Properties
  • Microscopes
  • Microscopy
  • Molecules
  • Optical Properties
  • Polymers
  • Surface Active Substances
  • Surface Tension

Fields of Study

  • Chemistry

Readers

  • Nanocomposite Materials Science
  • Petroleum Engineering
  • Thin Film Deposition Science.