Centimeter Wave Absorption in Molecular Crystals

Abstract

Molecular dynamics calculations performed at the University of Nebraska predict that temperature-dependent microwave activity is present in some ionic molecular crystals. This activity is due to the excitation of 'hindered rotations' or thermally activated 'hopping' modes for the molecular ions. Microwave reflectometer measurements performed at the BRL show temperature-dependent microwave losses occur in several ionic molecular crystals at or near the calculated order/disorder transition temperatures. These measurements, performed from 2 to 20 GHz from room temperature to about 300 deg C on the BRL 'arch,' were made on powder samples of the nitrates and nitrites of potassium, sodium, and other materials. Potassium nitrate displays an interesting temperature dependence with the absorption 'turning on' at about 1200 C, near the calculated order/disorder transition temperature. Measurements were also performed on selected ionic salts which uniformly show small microwave losses at any of the temperatures measured.

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Document Details

Document Type
Technical Report
Publication Date
Sep 01, 1992
Accession Number
ADA257453

Entities

People

  • Arthur Gauss Jr.
  • H. M. Lu
  • J. R. Hardy
  • Robert B. Bossoli
  • Steve G. Cornelison

Organizations

  • Ballistic Research Laboratory

Tags

Communities of Interest

  • Advanced Electronics
  • Space
  • Weapons Technologies

DTIC Thesaurus Topics

  • Absorption
  • Crystal Structure
  • Dipole Moments
  • Diseases And Disorders
  • Engineering
  • Materials
  • Measurement
  • Microwaves
  • Molecular Dynamics
  • Phase Transformations
  • Physics
  • Potassium
  • Reflectometers
  • Rotation
  • Sodium Compounds
  • Transition Temperature
  • Transitions

Fields of Study

  • Physics

Readers

  • Materials Science and Engineering.
  • Microwave Engineering.
  • Organic Chemistry