Electronic Control of pH at Sulfonated Polyaniline Electrodes

Abstract

The pH of aqueous solutions in the vicinity of a thin self-doped conducting polyaniline electrode was electrochemically modulated using both cyclic voltammetry and step potential techniques. Changes in pH were measured directly by using a microcombination pH probe. The experimental results demonstrate that the polymer behaves as a proton ejector during oxidation and a proton absorber during reduction. This potential-controlled pH change near the polymer coated electrode may be applied to many fields benefitting from electronic control of the proton environment near an electrode surface, for example, control of enzyme activity.

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Document Details

Document Type
Technical Report
Publication Date
Jul 01, 1992
Accession Number
ADA260074

Entities

People

  • Arthur J. Epstein
  • Jin Yue

Organizations

  • University of Pennsylvania

Tags

Communities of Interest

  • Materials and Manufacturing Processes

DTIC Thesaurus Topics

  • Abstracts
  • Aqueous Solutions
  • Chemical Engineering
  • Chemistry
  • Classification
  • Electrodes
  • Military Research
  • Monitoring
  • Oxidation
  • Pennsylvania
  • Photoelectrochemical Cells
  • Polyanilines
  • Polymers
  • Reaction Time
  • United States
  • Universities

Fields of Study

  • Materials science

Readers

  • Electrochemical Surface Science
  • Solar Physics

Technology Areas

  • Microelectronics