DN Hard Materials Laser Assisted Formation of Dense Phases

Abstract

Diamond and other high-pressure phases of carbon were synthesized in air by exposing fine particles of carbon black to carbon dioxide and Nd-YAG laser radiation. The high-pressure phases were separated from the carbon black by selective oxidation and were characterized by electron and x-ray diffraction. Formation of cubic diamond, chaoite, and graphite was confirmed. Exposure of a falling stream of 1 um average size a-quartz particles to a continuous wave or pulsed C02 laser beam in air resulted in the formation of a complete series of high-pressure phases of silica: coesite, stishovite, and apparently even denser forms with a-PbO2 and Fe2N structures. Since the laser exposure technique works with the carbon black to diamond transition, the technique is confirmed as a simple and generally applicable means to achieve the same effects as exposure to several hundred kilobars pressure. High-pressure phases of CaCO3, namely aragonite, calcite II, and possibly calcite III, were synthesized in air by exposing 10- to 20-um-size particles of CaCO3 (calcite I phase) to a C02 laser radiation at short pulse lengths (<O.l ms). The system B-0 was explored at high pressures and some very interesting new materials prepared near the composition B120-B220. The properties were not reproducible.... Diamond synthesis via laser pulses, Novel hard BxO phases.

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Document Details

Document Type
Technical Report
Publication Date
Jan 14, 1991
Accession Number
ADA262340

Entities

People

  • Roy Rustum

Organizations

  • Pennsylvania State University

Tags

Communities of Interest

  • Air Platforms
  • Energy and Power Technologies

DTIC Thesaurus Topics

  • Carbon Dioxide Lasers
  • Ceramic Materials
  • Chemical Reactions
  • Chemical Synthesis
  • Chemistry
  • Continuous Waves
  • Crystal Structure
  • Diffraction
  • High Pressure
  • Inorganic Chemistry
  • Laser Beams
  • Lasers
  • Materials
  • Materials Science
  • Phase Transformations
  • X Rays
  • X-Ray Diffraction

Fields of Study

  • Physics

Readers

  • Materials Science and Engineering.
  • Mathematics or Statistics
  • Pulsed Power and Plasma Physics.

Technology Areas

  • Directed Energy
  • Directed Energy - Pulsed-Laser Deposition
  • Microelectronics